Manager: E. T. J. Nibbering
Researchers: H. N. Ghosh
Ph.D. student: K. Adamczyk, M. Yang
Previous Researcher: G. Korn, M. Wittmann, A.
Kummrow, K. Heyne, A. Usman
Previous Ph.D. students: O. Dühr, F. Tschirschwitz,
M. Rini, O. F. Mohammed
Description
This laser set-up is dedicated to ultrafast experiments on
(bio-) molecular systems in the condensed phase. It consists of an
amplified 1 kHz/5 kHz Ti:sapphire system with frequency conversion
schemes from the near-UV via VIS and NIR to mid-IR, with detection
equipment dedicated for femtosecond mid-IR pump-probe and photon echo
experiments.
For more details on equipment see:
A. Kummrow et al., Appl. Phys. B 71 (2000), 885;
P. Hamm, R. A. Kaindl and J. Stenger, Opt. Lett. 25
(2000) 1798; M. Rini et al., Faraday Discuss. 122
(2003) 27; M. L . Cowan et al., Nature 434 (2005)
199.
For more details on applications see project
2-04.
Main projects (97/03)
1. Generation of Extremely Short Light Pulses
in the Violet-Blue and near Ultraviolet (MBI-Projekt 1.01)
G. Korn, E. T. J. Nibbering, O. Dühr, A. Kummrow, M. Wittmann,
F. Tschirschwitz (MBI)
G. Tempea, F. Krausz (TU Wien)
2. Intermolecular Hydrogen-Bonding Dynamics of
Coumarin Dyes in the Electronic Excited State
(MBI-Projekt 2.05; DFG-Schwerpunkt DFG-NI 492/2-1)
C. Chudoba, F. Tschirschwitz, E. T. J. Nibbering, T. Elsaesser (MBI)
3. Ultrafast Photochemistry of Chlorine Dioxide
in Solution
(MBI-Projekt 2.05; EU-Project MBI-97-005-01)
O. Dühr, F. Tschirschwitz, E. T. J. Nibbering (MBI)
H. Fidder (University of Uppsala)
4. Ultrafast Photochemistry of Chlorine Dioxide
in the Gas and Cluster Phase (MBI-Projekt 2.04)
V. Stert, H.-H. Ritze, E. T. J. Nibbering, W. Radloff (MBI)
5. Excited-State Intramolecular Proton Transfer
of 3-Hydroxyflavone (MBI-Projekt 2.05; EU-Project MBI-97-008-01)
E. T. J. Nibbering (MBI)
S. Ameer-Beg, S. M. Ormson, R. G. Brown (University of Central
Lancashire)
P. Matousek, M. Towrie (Rutherford Appleton Laboratory)
P. Foggi, F. V. R. Neuwahl (LENS)
6. Ultrafast Dynamics of Photosynthetic Reaction
Centra (MBI-Projekt 2.06; EU-Project)
F. Tschirschwitz, B. Voigt, J. Ehlert, E. T. J. Nibbering, D. Leupold,
T. Elsaesser (MBI)
L. Fiedor, H. Scheer (Botanisches Institut München)
C. N. Hunter (University of Sheffield)
7. Generation and Characterization of Femtosecond
Bessel Beams with Micro-Axicon Arrays (MBI-Projekt 1.03)
R. Grunwald, U. Griebner, F. Tschirschwitz, A. Kummrow, M. Rini,
E. T. J. Nibbering, T. Elsaesser (MBI)
V. Kebbel, H.-J. Hartmann, W. Jüptner (Bremer Institut
für Angewandte Strahltechnik (BIAS), Bremen)
8. Excited-State Intramolecular Hydrogen Transfer
Dynamics
(Projekt 2.05; DFG-Schwerpunkt DFG-NI 492/2-2)
M. Rini, A. Kummrow, J. Dreyer, E. T. J. Nibbering, T. Elsaesser
(MBI)
9. Excited-State Proton Transfer Dynamics of Photoacids
(Projekt 2.05; DFG-Schwerpunkt DFG-NI 492/2-2; EU-Project MBI000228)
M. Rini, A. Kummrow, J. Dreyer, E. T. J. Nibbering, T. Elsaesser
(MBI)
B.-Z. Magnes, E. Pines (Ben Gurion University, Beer-Sheva)
10. Two-photon excitation fluorescence spectrum
of the light harvesting complex LH2 from Chromatium minutissimum
between 650-745 nm
(Projekt 2.06; BMBF-WTZ RUS 99/174; RFBR 00-04-48308)
M. Krikunova, A. Kummrow, B. Voigt, M. Rini, D. Leupold (MBI)
H. Lokstein (Humboldt Universität)
H. Scheer (Botanisches Institut München)
A. Moskalenko, O. A. Toropygina (Russian Academy of Sciences)
A. Razjivin (M. V. Lomonosov Moscow State University)
11. Femtosecond Vibrational Studies of the Ring-Opening
Reaction Dynamics of Spiropyrans
(MBI-Projekt 2.05; EU-Project MBI000237)
M. Rini, E. T. J. Nibbering (MBI)
H. Fidder, A.-K. Holm (University of Uppsala)
12. CO and NO Geminate Recombination in Nitric
Oxide Synthase (NOS) Isoforms studied by Ultrafast Laser Photolysis
(MBI-Projekt 2.05; EU Project MBI000232)
M. Rini, K. Heyne, E. T. J. Nibbering (MBI)
T. Zemojtel (University of Gdansk; Universität Freiburg; Universität
Würzburg)
J. Scheele, T. Dandekar (Universität Freiburg)
V. Sharma (University of California at San Diego, La Jolla, California)
P. Kozlowski (University of Louisville, Kentucky)
13. Dynamics of Ligand Exchange in Ru(dcbpy)(CO)2I2
(MBI-Projekt 2.05; EU Project MBI000290)
M. Rini, E. T. J. Nibbering (MBI)
V. Lehtovuori, J. Korppi-Tommola (University of Jyvaskyla)
14. Excited-State Dynamics of Chromophores of
Green Fluorescent Protein
(MBI-Projekt 2-04)
O. F. Mohammed, A. Usman, E. T. J. Nibbering (MBI)
J. Dong, K. Solntsev, L. M. Tolbert (Georgia Institute of Technology,
Atlanta)
15. Structural Dynamics of Photoactive Yellow
Protein
(MBI-Projekt 2-04)
O. F. Mohammed, A. Usman, K. Heyne, J. Dreyer, E. T. J. Nibbering
(MBI)
M. A. Cusanovich (University of Arizona at Tucson)
16. Photoinduced Bimolecular Electron Transfer
(MBI-Projekt 2-04; EU Project MBI001176)
O. F. Mohammed, K. Adamczyk, J. Dreyer, E. T. J. Nibbering (MBI)
O. F. Mohammed, N. Banerji, B. Lang, E. Vauthey (University of Geneva)
for contact click here:
E. T. J. Nibbering
Pictures
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Hirendra N. Ghosh (MBI/BARC) (October 2007) |
 |
Bernhard Lang (University of Geneva), Omar
F. Mohammed (MBI/University of Geneva), Erik T. J. Nibbering
(MBI) and Natalie Banerji (University of Geneva) (July 2005) |
 |
Omar F. Mohammed and Katrin Adamczyk (MBI)
(March 2005) |
|
Matteo Rini (MBI), Henk Fidder (University
of Uppsala) and Omar F.Mohammed |
 |
Matteo Rini (MBI) and Tomasz Zemojtel (Universität
Freiburg) (July 2002) |
 |
Volker Kebbel (BIAS/Bremen) (December
2001) |
 |
Andreas Kummrow and Matteo Rini (MBI) (August
2000) |
 |
Frank Tschirschwitz (MBI) and Henk
Fidder (University of Uppsala) (November 1998) |
 |
Frank Tschirschwitz and Oliver Dühr
(MBI) (August 1998) |
 |
Georg Korn, Erik T. J. Nibbering and Oliver
Dühr (MBI) (April 1997) |
 |
Oliver Dühr (MBI) (April 1997)
|
 |
Erik T. J. Nibbering (MBI) (January
1997) |
 |
Oliver Dühr and Georg Korn (MBI)
(September 1996) |
Specifications
|
|
|
| Fundamental |
Amplified Ti:sapphire laser system @ 800 nm (pulse energy
5 mJ @ 1 kHz or 1 mJ @ 5 kHz, pulse duration 45 fs) |
| Second harmonic |
50fs, 20µJ@400nm |
| VIS |
Noncollinear optical parametric
amplifier stage for tunable visible pulses (spectral range 480-660
nm; pulse energy 1 µJ; pulse duration 50 fs) |
| near-UV |
Frequency conversion scheme
for tunable near-UV pulses (spectral range 310-360 nm; pulse
energy 1 µJ; pulse duration 50 fs) |
| mid-IR |
Parametric down-conversion
scheme for tunable mid-IR pulses (spectral range 2-20 µm;
pulse energy 0.3-1 µJ; pulse duration 100 fs). |
Special detection system
|
Monochromator-mid-IR diode
array enabling frequency-resolved detection of the mid-infrared. |
| Experimental Set-Ups |
UV/vis-IR pump-probe;
IR-pump-probe; IR heterodyne-detected photon echo set-up |
|